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Comparison of different valent iron on anaerobic sludge digestion: Focusing on oxidation reduction potential

《环境科学与工程前沿（英文）》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1514-3

摘要：

• ORP value from −278.71 to −379.80 mV showed indiscernible effects on methane yield.

关键词： Enhanced anaerobic sludge digestion     Different iron valence     Oxidation reduction potential     Dissolved organic nitrogen     Microbial community    

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Revealing the GHG reduction potential of emerging biomass-based CO utilization with an iron cycle system

《环境科学与工程前沿（英文）》 2023年 第17卷 第10期 doi: 10.1007/s11783-023-1727-8

摘要：

● Greenhouse gas mitigation by biomass-based CO2 utilization with a Fe cycle system.

关键词： Carbon dioxide utilization     Hydrothermal reactions     Biomass-based CO2 reduction     Simulation     Ex-ante LCA    

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Reduction potential of the energy penalty for CO capture in CCS

《能源前沿（英文）》 2023年 第17卷 第3期   页码 390-399 doi: 10.1007/s11708-023-0864-x

摘要： CO2 capture and storage (CCS) has been acknowledged as an essential part of a portfolio of technologies that are required to achieve cost-effective long-term CO2 mitigation. However, the development progress of CCS technologies is far behind the targets set by roadmaps, and engineering practices do not lead to commercial deployment. One of the crucial reasons for this delay lies in the unaffordable penalty caused by CO2 capture, even though the technology has been commonly recognized as achievable. From the aspects of separation and capture technology innovation, the potential and promising direction for solving this problem were analyzed, and correspondingly, the possible path for deployment of CCS in China was discussed. Under the carbon neutral target recently proposed by the Chinese government, the role of CCS and the key milestones for deployment were indicated.

关键词： CO2 capture and storage (CCS)     CO2 separation     energy penalty    

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China’s pre-2020 CO

Hailin WANG

《能源前沿（英文）》 2019年 第13卷 第3期   页码 571-578 doi: 10.1007/s11708-019-0640-0

摘要： China achieved the reduction of CO intensity of GDP by 45% compared with 2005 at the end of 2017, realizing the commitment at 2009 Copenhagen Conference on emissions reduction 3 years ahead of time. In future implementation of the “13th Five-Year Plan (FYP),” with the decline of economic growth rate, decrease of energy consumption elasticity and optimization of energy structure, the CO intensity of GDP will still have the potential for decreasing before 2020. By applying KAYA Formula decomposition, this paper makes the historical statistics of the GDP energy intensity decrease and CO intensity of energy consumption since 2005, and simulates the decrease of CO intensity of GDP in 2020 and its influences on achieving National Determined Contribution (NDC) target in 2030 with scenario analysis. The results show that China’s CO intensity of GDP in 2020 is expected to fall by 52.9%–54.4% than the 2005 level, and will be 22.9%–25.4% lower than 2015. Therefore, it is likely to overfulfill the decrease of CO intensity of GDP by 18% proposed in the 13th FYP period. Furthermore, the emission reduction potentiality before 2020 will be conducive to the earlier realization of NDC objectives in 2030. China’s CO intensity of GDP in 2030 will fall by over 70% than that in 2005, and CO emissions peak will appear before 2030 as early as possible. To accelerate the transition to a low-carbon economy, China needs to make better use of the carbon market, and guide the whole society with carbon price to reduce emissions effectively. At the same time, China should also study the synergy of policy package so as to achieve the target of emission reduction.

关键词： China’s National Determined Contribution     emission reduction potential     scenario analysis     CO2 emissions peak    

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Advanced nitrogen removal by pulsed sequencing batch reactors (SBR) with real-time control

YANG Qing, PENG Yongzhen, YANG Anming, LI Jianfeng, GUO Jianhua

《环境科学与工程前沿（英文）》 2007年 第1卷 第4期   页码 488-492 doi: 10.1007/s11783-007-0078-1

摘要： The feasibility of pH and oxidation reduction potential (ORP) as on-line control parameters to advance nitrogen removal in pulsed sequencing batch reactors (SBR) was evaluated. The pulsed SBR, a novel operational mode of SBR, was

关键词： reduction potential     oxidation reduction     operational     feasibility     nitrogen    

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Scenario analysis of the energy demand and CO

Jihong ZHANG, Jian ZHOU, Guangping HU, Tianhou ZHANG

《能源前沿（英文）》 2010年 第4卷 第4期   页码 459-468 doi: 10.1007/s11708-010-0119-5

摘要： An assessment of the energy demand and the potential for sector-based emission reductions will provide necessary background information for policy makers. In this paper, Beijing was selected as a special case for analysis in order to assess the energy demand and potential of CO abatement in the urban transport system of China. A mathematical model was developed to generate three scenarios for the urban transport system of Beijing from 2010 to 2030. The best pattern was identified by comparing the three different scenarios and assessing their urban traffic patterns through cost information. Results show that in the high motorization-oriented pattern scenario, total energy demand is about 13.94% higher, and the average CO abatement per year is 3.38 million tons less than in the reference scenario. On the other hand, in the bus and rail transit-oriented scenario, total energy demand is about 11.57% less, and the average CO abatement is 2.8 million tons more than in the reference scenario. Thus, Beijing cannot and should not follow the American pattern of high motorization-oriented transport system but learn from the experience of developed cities of Europe and East Asia.

关键词： scenario analysis     urban traffic pattern     energy demand     reduction potential    

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New insight into effect of potential on degradation of Fe-N-C catalyst for ORR

Yanyan GAO, Manman QI, Liang HE, Haiping CHEN, Wenzhe LUO, Ming HOU, Zhigang SHAO

《能源前沿（英文）》 2021年 第15卷 第2期   页码 421-430 doi: 10.1007/s11708-021-0727-2

摘要： In recent years, Fe-N-C catalyst is particularly attractive due to its high oxygen reduction reaction (ORR) activity and low cost for proton exchange membrane fuel cells (PEMFCs). However, the durability problems still pose challenge to the application of Fe-N-C catalyst. Although considerable work has been done to investigate the degradation mechanisms of Fe-N-C catalyst, most of them are simply focused on the active-site decay, the carbon oxidation, and the demetalation problems. In fact, the 2e pathway in the ORR process of Fe-N-C catalyst would result in the formation of H O , which is proved to be a key degradation source. In this paper, a new insight into the effect of potential on degradation of Fe-N-C catalyst was provided by quantifying the H O intermediate. In this case, stability tests were conducted by the potential-static method in O saturated 0.1 mol/L HClO . During the tests, H O was quantified by rotating ring disk electrode (RRDE). The results show that compared with the loading voltage of 0.4 V, 0.8 V, and 1.0 V, the catalysts being kept at 0.6 V exhibit a highest H O yield. It is found that it is the combined effect of electrochemical oxidation and chemical oxidation (by aggressive radicals like H O /radicals) that triggered the highest H O release rate, with the latter as the major cause.

关键词： proton exchange membrane fuel cells (PEMFCs)     oxygen reduction reaction (ORR)     Fe-N-C catalyst     potential     H2O2     degradation    

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doped carbon nanotubes encapsulating M(Co, Fe)-Ni alloy for electrochemical production of syngas with potential-independent

《化学科学与工程前沿（英文）》 2022年 第16卷 第4期   页码 498-510 doi: 10.1007/s11705-021-2082-6

摘要： The electrochemical conversion of CO2-H2O into CO-H2 using renewable energy is a promising technique for clean syngas production. Low-cost electrocatalysts to produce tunable syngas with a potential-independent CO/H2 ratio are highly desired. Herein, a series of N-doped carbon nanotubes encapsulating binary alloy nanoparticles (MxNi-NCNT, M= Fe, Co) were successfully fabricated through the co-pyrolysis of melamine and metal precursors. The MxNi-NCNT samples exhibited bamboo-like nanotubular structures with a large specific surface area and high degree of graphitization. Their electrocatalytic performance for syngas production can be tuned by changing the alloy compositions and modifying the electronic structure of the carbon nanotube through the encapsulated metal nanoparticles. Consequently, syngas with a wide range of CO/H2 ratios, from 0.5:1 to 3.4:1, can be produced on MxNi-NCNT. More importantly, stable CO/H2 ratios of 2:1 and 1.5:1, corresponding to the ratio to produce biofuels by syngas fermentation, could be realized on Co1Ni-NCNT and Co2Ni-NCNT, respectively, over a potential window of –0.8 to –1.2 V versus the reversible hydrogen electrode. Our work provides an approach to develop low-cost and potential-independent electrocatalysts to effectively produce syngas with an adjustable CO/H2 ratio from electrochemical CO2 reduction.

关键词： electrochemical reduction of CO2     syngas     N-doped carbon nanotubes     encapsulated alloy nanoparticles     CO/H2 ratio    

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Effect of environment change on the strength of cement/lime treated clays

Takenori HINO, Rui JIA, Seiji SUEYOSHI, Tri HARIANTO

《结构与土木工程前沿（英文）》 2012年 第6卷 第2期   页码 153-165 doi: 10.1007/s11709-012-0153-y

摘要： The field strengths of cement/lime treated clays were investigated in the Ariake Sea costal lowlands. The deposition environment of the investigation location is reconstructed and compared to the present ground environment. The mechanism of the ground environment change and its effect on the strength of cement/lime treated soil are discussed. The strength development of improved soil using cement and lime in different curing environments was investigated in the laboratory for studying the effect of environment change on the strength also. It has been found that the strength deterioration of improved soil in deep mixing method is due to 1) the ground environment change due to the secondary oxidation which results in low pH value and high organic content, and 2) the formations of the porous structures result from the elution of the calcium ions. Also, it has been found that the initial strength increase of the improved soil is related to the dissolved silica and that the dissolution of the silica in clay minerals needs long time. When examining the long-term strength for preventing strength degradation, the effect of environmental change has to be considered. The importance of measuring pH and oxidation-reduction potential (ORP) of the ground for cement/lime solidification method is explained.

关键词： soil solidification     ground environment     strength deterioration     pH     oxidation-reduction potential (ORP)     silica    

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Thermochemical pretreatment of meat and bone meal and its effect on methane production

Guangxue WU , Zhenhu HU , Mark G. HEALY , Xinmin ZHAN ,

《环境科学与工程前沿（英文）》 2009年 第3卷 第3期   页码 300-306 doi: 10.1007/s11783-009-0031-6

摘要： Since the solubilization of meat and bone meal (MBM) is a prerequisite in many MBM disposal approaches, enhancement of the solubilization by means of thermochemical pretreatment was investigated in this study at two temperatures (55°C and 131°C) and six sodium hydroxide (NaOH) concentrations (0, 1.25, 2.5, 5, 10 and 20g/L). The MBM volatile solid (VS) reduction ratio was up to 66% and 70% at 55°C and 131°C, respectively. At the same temperature, the VS reduction ratio increased with the increase in the dosage of NaOH. The study on the methane (CH) production potential of pretreated MBM shows that the addition of NaOH at 55°C did not cause the inhibition of the succeeding CH production process. However, CH production was inhibited by the addition of NaOH at 131°C. The CH production potential was in the range of 389 to 503mL CH/g VS MBM and 464 to 555mL CH/g VS MBM at 55°C and 131°C, respectively.

关键词： thermochemical pretreatment     meat and bone meal     solid reduction     solid solubilization     methane production potential    

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Novel coprecipitation–oxidation method for recovering iron from steel waste pickling liquor

Shejiang Liu, Hongyang Yang, Yongkui Yang, Yupeng Guo, Yun Qi

《环境科学与工程前沿（英文）》 2017年 第11卷 第1期 doi: 10.1007/s11783-017-0902-1

摘要： Coprecipitation–oxidation method was developed to recover the iron from wastewater. Fe O nanoparticles were well synthesized from steel waste pickling liquor. Promoters greatly improved the properties of synthesized Fe O nanoparticle. Real-time control of the Fe /Fe molar ratio was achieved by ORP monitoring. Waste pickling liquors (WPLs) containing high concentrations of iron and acid are hazardous waste products from the steel pickling processes. A novel combined coprecipitation–oxidation method for iron recovery by Fe O nanoparticle production from the WPLs was developed in this study. An oxidation–reduction potential monitoring method was developed for real-time control of the Fe /Fe molar ratio. The key coprecipitation–oxidation parameters were determined using the orthogonal experimental design method. The use of promoters greatly improved the Fe O nanoparticle crystallinity, size, magnetization, and dispersion. X-ray diffraction patterns showed that the produced Fe O nanoparticles were single phase. The Fe O nanoparticles were approximately spherical and slightly agglomerated. Vibrating sample magnetometry showed that the Fe O nanoparticles produced from the WPLs had good magnetic properties, with a saturation magnetization of 80.206 emu·g and a remanence of 10.500 emu·g . The results show that this novel coprecipitation–oxidation method has great potential for recycling iron in WPLs.

关键词： Waste pickling liquor     Coprecipitation–oxidation     Fe3O4 nanoparticles     Oxidation–reduction potential     Promoter    

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我国碳捕集利用与封存技术发展研究

张贤,李阳,马乔,刘玲娜

《中国工程科学》 2021年 第23卷 第6期   页码 70-80 doi: 10.15302/J-SSCAE-2021.06.004

摘要：

碳捕集利用与封存（ CCUS）是实现碳中和目标不可或缺的重要技术选择。为了系统梳理技术发展现状、明确未来发展方向，本文对我国 CCUS 技术水平、示范进展、成本效益、潜力需求等进行了全面评估。我国 CCUS 技术发展迅速，与国际整体发展水平相当，目前处于工业化示范阶段，但部分关键技术落后于国际先进水平。在工业示范方面，我国具备了大规模捕集利用与封存的工程能力，但在项目规模、技术集成、海底封存、工业应用等方面与国际先进水平还存在差距。在减排潜力与需求方面，我国理论封存容量和行业减排需求极大，考虑源汇匹配之后不同地区陆上封存潜力差异较大。在成本效益方面，尽管当前 CCUS 技术成本较高，但未来可有效降低实现碳中和目标的整体减排成本。为此建议，加快构建 CCUS 技术体系，推进全链条集成示范，加快管网布局和基础设施建设，完善财税激励政策和法律法规体系。

关键词： 碳中和，CCUS，技术研发与示范，减排潜力，成本与效益    

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Trophic mode and organics metabolic characteristic of fungal community in swine manure composting

Jing Peng, Ke Wang, Xiangbo Yin, Xiaoqing Yin, Mengfei Du, Yingzhi Gao, Philip Antwi, Nanqi Ren, Aijie Wang

《环境科学与工程前沿（英文）》 2019年 第13卷 第6期 doi: 10.1007/s11783-019-1177-5

摘要： Fungal trophic modes and substrates utilization ability was observed in composting. Fungi had the higher diversity and more trophic types in thermophilic phase. Fungi had the higher metabolic potential in fresh swine manure and mature production. Redox potential, organics and moisture are main factors impacting fungal community. Composting reduced pathogenic fungi and enrich dung saprotroph fungi in swine manure. The succession of fungal community, trophic mode and metabolic characteristics were evaluated in 60 days composting of swine manure by high-throughput sequencing, FUNGuild and Biolog method, respectively. The result showed that the fungal community diversity reached to the highest level (76 OTUs) in the thermophilic phase of composting, then sustained decline to 15 OTUs after incubation. There were 10 fungal function groups in the raw swine manure. Pathotroph-saprotroph fungi reached to 15.91% on Day-10 but disappeared on Day-60. Dung saprotroph-undefined saprotroph fungi grown from 0.19% to 52.39% during the treatment. The fungal community had more functional groups but the lower substrate degradation rates in the thermophilic phase. The fungal communities on Day-0 and Day-60 had the highest degradation rates of amino acids and polymers, respectively. Redundancy analysis showed that ORP (49.6%), VS/Ash (45.3%) and moisture (39.2%) were the main influence factors on the succession of fungal community in the swine manure composting process.

关键词： Fungus     FUNGuild     Biolog     Trophic mode     Composting     Oxidation reduction potential    

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电解锰行业污染防治最佳可行技术评估及污染减排潜力

李旭华,方刚,党春阁,于秀玲

《中国工程科学》 2013年 第15卷 第3期   页码 56-61

摘要：

电解锰行业废水排放量大，污染物浓度高，属于高污染行业，是我国实现污染物控制减排的主要威胁之一。通过对电解锰行业污染防治现状进行分析，构建了污染防治技术评估指标体系，利用层次分析法确定各评价指标的权重，利用综合评价值法对电解锰行业污染防治技术进行了评估。在此基础上，利用自底向上模型对评估出的最佳可行技术的污染减排潜力进行预测。结果表明，与基准年2010年相比，2015年电解锰行业废水排放总量可削减270多万吨，氨氮减排6.6×104 t，减排回收的锰和重铬酸钾可分别达到1.9×105 t和3.747×107 t，锰渣减排4×106 t；同时也表明清洁生产技术减排的能力高于末端治理技术减排，清洁生产技术具有较大的推广普及潜力。

关键词： 电解锰     污染防治     最佳可行技术     减排     潜力    

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Energy neutrality potential of wastewater treatment plants: A novel evaluation framework integrating

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1549-0

摘要：

• Framework of indicators was established based on energy efficiency and recovery.

关键词： Wastewater treatment plants     Energy neutrality potential     Energy efficiency     Energy recovery     Evaluation framework    

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标题 作者 时间 类型 操作

Comparison of different valent iron on anaerobic sludge digestion: Focusing on oxidation reduction potential

期刊论文

Revealing the GHG reduction potential of emerging biomass-based CO utilization with an iron cycle system

期刊论文

Reduction potential of the energy penalty for CO capture in CCS

期刊论文

China’s pre-2020 CO

Hailin WANG

期刊论文

Advanced nitrogen removal by pulsed sequencing batch reactors (SBR) with real-time control

YANG Qing, PENG Yongzhen, YANG Anming, LI Jianfeng, GUO Jianhua

期刊论文

Scenario analysis of the energy demand and CO

Jihong ZHANG, Jian ZHOU, Guangping HU, Tianhou ZHANG

期刊论文

New insight into effect of potential on degradation of Fe-N-C catalyst for ORR

Yanyan GAO, Manman QI, Liang HE, Haiping CHEN, Wenzhe LUO, Ming HOU, Zhigang SHAO

期刊论文

doped carbon nanotubes encapsulating M(Co, Fe)-Ni alloy for electrochemical production of syngas with potential-independent

期刊论文

Effect of environment change on the strength of cement/lime treated clays

Takenori HINO, Rui JIA, Seiji SUEYOSHI, Tri HARIANTO

期刊论文

Thermochemical pretreatment of meat and bone meal and its effect on methane production

Guangxue WU , Zhenhu HU , Mark G. HEALY , Xinmin ZHAN ,

期刊论文

Novel coprecipitation–oxidation method for recovering iron from steel waste pickling liquor

Shejiang Liu, Hongyang Yang, Yongkui Yang, Yupeng Guo, Yun Qi

期刊论文

我国碳捕集利用与封存技术发展研究

张贤,李阳,马乔,刘玲娜

期刊论文

Trophic mode and organics metabolic characteristic of fungal community in swine manure composting

Jing Peng, Ke Wang, Xiangbo Yin, Xiaoqing Yin, Mengfei Du, Yingzhi Gao, Philip Antwi, Nanqi Ren, Aijie Wang

期刊论文

电解锰行业污染防治最佳可行技术评估及污染减排潜力

李旭华,方刚,党春阁,于秀玲

期刊论文

Energy neutrality potential of wastewater treatment plants: A novel evaluation framework integrating

期刊论文